Download Adsorption on Surfaces and Surface Diffusion of Adsorbates by E.I. Altman, M. Bienfait, H.P. Bonzel, R. Diehl, M.Y.L. PDF

By E.I. Altman, M. Bienfait, H.P. Bonzel, R. Diehl, M.Y.L. Jung, V.G. Lifshitz, M.E. Michel, R. Miranda, R. McGrath, K. Oura, A.A. Saranin, E.G. Seebauer, P. Zeppenfeld, A.V. Zotov

Floor technological know-how is known as a comparatively younger medical self-discipline, curious about the actual and chemical houses of and phenomena on fresh and lined good surfaces, studied below a number of stipulations. The adsorption of atoms and molecules on stable surfaces is, for instance, this sort of situation, hooked up with roughly drastic adjustments of all floor homes. An adsorption occasion is usually saw in nature and located to be of technical value in lots of commercial tactics. therefore, floor technology is interdisciplinary by means of its very nature, and as such a major middleman among basic and utilized learn. the current quantity forty two is dedicated to lined stable Surfaces and, specifically, Subvolume A to Adsorbed Layers on Surfaces. it truly is as any such number of facts received for adsorbates on well-defined crystalline surfaces. "Well-defined" skill surfaces of recognized crystallographic constitution and chemical composition.

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Extra info for Adsorption on Surfaces and Surface Diffusion of Adsorbates (Landolt-Börnstein: Numerical Data and Functional Relationships in Science and Technology - New Series Condensed Matter)

Example text

Gas temperature is 300 K, surface temperature 190 K [85Ste]. 7 for CO and H2 on a Ni(111) surface [84Ste, 85Rob, 85Ste]. In both cases the angular adsorption and desorption rates are clearly the same, confirming first of all the validity of detailed balancing and hence a quasi-equilibrium situation. Secondly, an excellent cosine distribution is found in the case of CO, in agreement with Eq. (27) and consistent with the sticking coefficient being close to unity for CO on Ni(111) [74Chr, 80Iba]. e.

However, an effect interfering with this useful correlation between core electron binding energy and chemical/physical state of the adsorbed species is the electronic screening of the hole generated by the photoemission process [82Sie]. The hole screening effects the kinetic energy of the departing photoelectron and hence its apparent binding energy. This final state effect therefore influences the measured electron binding energy in a way that is not straightforwardly associated with the local substrate-adsorbate bond.

A) upper part: experimental data, 2-fold averaged, (b) lower part: single scattering calculation [98Emu]. Angle-resolved XPD measurements of C1s intensities from the well ordered (2×1)p2mg-CO layer over a large solid angle are in good agreement with the structure model [75Lam]. Figure 14 showed already four C1s peaks for the [001] azimuth in a single polar angle scan. If the C1s intensity is recorded for the same layer over a large solid angle, other forward scattering peaks arising from intermolecular Landolt-Börnstein New Series III/42A Ref.

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